Robert Mitchum as Max Cady in Cape Fear
Douglas Rain (voice) as HAL 9000 in 2001: A Space Odyssey
Dennis Hopper as Frank Booth in Blue Velvet
Orson Welles as Hank Quinlan in Touch of Evil
Carl Boehm as Mark Lewis in Peeping Tom
Lee Marvin as Liberty Valance in The Man Who Shot Liberty Valance
R. Lee Ermey as Gunnery Sergeant Hartman in Full Metal Jacket
Gary Oldman as Norman Stansfield in Leon
Joseph Cotton as Uncle Charlie in Shadow Of A Doubt
Gunnar Hansen as Leatherface in The Texas Chainsaw Massacre
Barbara Stanwyck as Phyllis Dietrichson in Double Indemnity
Christopher Walken as Vincenzo Coccotti in True Romance
Christoph Waltz as Hans Landa in Inglorious Basterds
Orson Welles as Harry Lime in The Third Man
A Moose Head as The Moose Head in Evil Dead II: Dead by Dawn
...but my favourite is Lee Van Cleef as Angel Eyes in The Good, The Bad & The Ugly
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